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2D Co-Directed Metal–Organic Networks Featuring Strong Antiferromagnetism and Perpendicular Anisotropy

Identificadores del recurso

Small 20.22 (2023): 2309555

1613-6810

http://hdl.handle.net/10486/713177

10.1002/smll.202309555

2309555-1

2309555-9

Procedència

(Biblos-e Archivo)

Fitxa

Títol:: 2D Co-Directed Metal–Organic Networks Featuring Strong Antiferromagnetism and Perpendicular Anisotropy
Tema:: X-ray magnetic circular dichroism; antiferromagnetism; cobalt; metal–organic network; scanning tunneling microscopy; perpendicular anisotropy; Física
Descripció:: Antiferromagnetic spintronics is a rapidly emerging field with the potential to revolutionize the way information is stored and processed. One of the key challenges in this field is the development of novel 2D antiferromagnetic materials. In this paper, the first on-surface synthesis of a Co-directed metal–organic network is reported in which the Co atoms are strongly antiferromagnetically coupled, while featuring a perpendicular magnetic anisotropy. This material is a promising candidate for future antiferromagnetic spintronic devices, as it combines the advantages of 2D and metal–organic chemistry with strong antiferromagnetic order and perpendicular magnetic anisotropy; S.O.P. and C.M.-F. contributed equally to this work. This work received funding from the European Research Council (ERC, grant 766555), Marie Sklodowska-Curie Actions (MSCA, project 894924) under the European Union’s Horizon 2020 Research and Innovation Programme, and the EMPIR Programme co-financed by the Participating States and the European and Union’s Horizon 2020 Research and Innovation Programme (grant EMPIR 20FUN03 COMET). IMDEA Nanociencia acknowledges financial support from the Spanish Ministry of Science and Innovation “Severo Ochoa” (Grant CEX2020-001039-S). The ALBA synchrotron is acknowledged for providing beam time at BOREAS beamline (proposal number 2021025046). JIM acknowledges funding by Spanish MICINN (Grants PID2020-113142RB-C21 and PLEC2021-007906, funded by MCIN/AEI/10.13039/501100011033, and TED2021-129416A I00 funded by MCIN/AEI/10.13039/501100011033 and EU NextGeneration EU/PRTR), and Comunidad de Madrid (Grants S2018/NMT-4367 and Y2020/NMT-6469). M.A.V. and B.M.C. acknowledge support from Spanish Ministry of Science and Innovation (MICINN) and the Spanish Research Agency MICIN/AEI through Project PID2021-123776NB-C21 (CONPHASETM)
Idioma:: English
Relació:: Gobierno de España. CEX2020-001039-S; Gobierno de España. PID2020-113142RB-C21; Gobierno de España. PLEC2021-007906; Gobierno de España. TED2021-129416A I00; Gobierno de España. PID2021-123776NB-C21; Comunidad de Madrid. S2018/NMT-4367; Comunidad de Madrid. Y2020/NMT-6469
Autor/Productor:: Parreiras, Sofía O.; Martín Fuentes, María; Moreno, Daniel; Mathialagan, Shanmugasibi K.; Biswas, Kalyan; Muñíz-Cano, Beatriz; Lauwaet, Koen; Valvidares, Manuel; Valbuena, Miguel A.; Urgel, José I.; Gargiani, Pierluigi; Camarero, Julio; Miranda, Rodolfo; Martínez, José I.; Gallego, José M.; Écija, David
Editor:: John Wiley and Sons Inc
Drets:: http://creativecommons.org/licenses/by/4.0/; open access
Data:: 2023-01-01
Tipo de recurso:: journal article; info:eu-repo/semantics/publishedVersion
Format:: application/pdf

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2. <dc:creator>Parreiras, Sofía O.</dc:creator>
3. <dc:creator>Martín Fuentes, María</dc:creator>
4. <dc:creator>Moreno, Daniel</dc:creator>
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19. <dc:subject>antiferromagnetism</dc:subject>
20. <dc:subject>cobalt</dc:subject>
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22. <dc:subject>scanning tunneling microscopy</dc:subject>
23. <dc:subject>perpendicular anisotropy</dc:subject>
24. <dc:subject>Física</dc:subject>
25. <dc:description>Antiferromagnetic spintronics is a rapidly emerging field with the potential to revolutionize the way information is stored and processed. One of the key challenges in this field is the development of novel 2D antiferromagnetic materials. In this paper, the first on-surface synthesis of a Co-directed metal–organic network is reported in which the Co atoms are strongly antiferromagnetically coupled, while featuring a perpendicular magnetic anisotropy. This material is a promising candidate for future antiferromagnetic spintronic devices, as it combines the advantages of 2D and metal–organic chemistry with strong antiferromagnetic order and perpendicular magnetic anisotropy</dc:description>
26. <dc:description>S.O.P. and C.M.-F. contributed equally to this work. This work received funding from the European Research Council (ERC, grant 766555), Marie Sklodowska-Curie Actions (MSCA, project 894924) under the European Union’s Horizon 2020 Research and Innovation Programme, and the EMPIR Programme co-financed by the Participating States and the European and Union’s Horizon 2020 Research and Innovation Programme (grant EMPIR 20FUN03 COMET). IMDEA Nanociencia acknowledges financial support from the Spanish Ministry of Science and Innovation “Severo Ochoa” (Grant CEX2020-001039-S). The ALBA synchrotron is acknowledged for providing beam time at BOREAS beamline (proposal number 2021025046). JIM acknowledges funding by Spanish MICINN (Grants PID2020-113142RB-C21 and PLEC2021-007906, funded by MCIN/AEI/10.13039/501100011033, and TED2021-129416A I00 funded by MCIN/AEI/10.13039/501100011033 and EU NextGeneration EU/PRTR), and Comunidad de Madrid (Grants S2018/NMT-4367 and Y2020/NMT-6469). M.A.V. and B.M.C. acknowledge support from Spanish Ministry of Science and Innovation (MICINN) and the Spanish Research Agency MICIN/AEI through Project PID2021-123776NB-C21 (CONPHASETM)</dc:description>
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